MRS Meetings and Events

 

QM01.02.01 2023 MRS Spring Meeting

Skyrmionics and Meronics Based on Inversion Symmetric Layered Ferromagnets

When and Where

Apr 11, 2023
1:30pm - 2:00pm

Marriott Marquis, Fourth Level, Pacific A

Presenter

Co-Author(s)

Luis Balicas1,2

Florida State Univ1,National High Magnetic Field Lab2

Abstract

Luis Balicas1,2

Florida State Univ1,National High Magnetic Field Lab2
Here, we will discuss the role of topological spin textures on the electrical and thermal transport properties of layered ferromagnets like Fe<sub>3-x</sub>GeTe<sub>2</sub> and Fe<sub>5-x</sub>GeTe<sub>2</sub>. In Fe<sub>3-x</sub>GeTe<sub>2</sub>, a layered ferromagnetic displaying a Curie temperature <i>T</i><sub>c</sub> ≈ 220 K, we observe[1] anomalous transport variables for magnetic fields m<sub>0</sub><i>H</i> applied along the gradient of the chemical potential generated by thermal gradients or electrical currents, a configuration that should not lead to their observation due to the absence of Lorentz force. These anomalous planar quantities are found to not scale with the component of the planar magnetization (<i>M</i><sub>||</sub>), showing instead a sharp decrease beyond m<sub>0</sub><i>H</i><sub>||</sub> = 4 T which is the field required to align the magnetic moments along m<sub>0</sub><i>H</i>||. We argue that locally chiral spin structures, such as skyrmions, and probably hybrid domain walls, lead to a field dependent spin-chirality. This in turn generates a novel type of topological transport in the absence of interaction between the magnetic field and electrical or thermal currents. For Fe<sub>5-x</sub>GeTe<sub>2</sub> (<i>T</i><sub>c</sub> ≈ 310-330 K) this unconventional topological transport is observed at, and beyond room temperature, correlating with the observation of merons through Lorentz transmission electron microscopy (LTEM)[2]. LTEM in Fe<sub>5-x</sub>GeTe<sub>2</sub> also reveals the coexistence of merons with skyrmions upon approaching its magnetostructural transition at <i>T</i><sub>s</sub> ≈ 110 K, due to a progressive rotation of the magneto-crystalline axial anisotropy towards the c-axis. The presence of these spin textures and their coexistence is exposed by thermal transport measurements as a function of the temperature, which unveils, for example, an anomalously large Nernst effect. Therefore, in Fe<sub>5-x</sub>GeTe<sub>2</sub> the formation and stabilization of distinct thermally driven topological spin textures can be chosen on demand by just adjusting the temperature. Given that Fe<sub>5-x</sub>GeTe<sub>2</sub> can be grown in large area substrates and its Ni and Co doped crystals display <i>T</i><sub>c</sub>s well above room temperature, we suggest that this compound along with its doped variants, can, not only open a new era in skyrmionics, but also open a new field of research, that of meronics.<br/><br/>[1] J. Macy <i>et al</i>., Appl. Phys. Rev. <b>8</b>, 041401 (2021).<br/>[2] B. Casas <i>et al</i>., (under review).

Keywords

2D materials | magnetic properties | thermal conductivity

Symposium Organizers

Kostya Novoselov, National University of Singapore
Elton Santos, University of Edinburgh
Srinivasa Rao Singamaneni, The University of Texas at El Paso
Michael Susner, Air Force Research Laboratory

Symposium Support

Platinum
National Science Foundation

Gold
Army Research Office

Bronze
QUANTUM DESIGN

Publishing Alliance

MRS publishes with Springer Nature