MRS Meetings and Events

 

QT01.05.07 2024 MRS Spring Meeting

Dynamic Control of Macroscopic Phases via Thermal Quench in 1T-TaS2

When and Where

Apr 24, 2024
3:30pm - 4:00pm

Room 420, Level 4, Summit

Presenter

Co-Author(s)

Alberto De la Torre1

Northeastern University1

Abstract

Alberto De la Torre1

Northeastern University1
In materials with competing order parameters, quenching across a phase transition can lead to the system being trapped in a long-lived metastable phase, even if it is not the global free-energy minimum. Examples of this phenomenology can be found over multiple energies and length scales - from the evolution of the known Universe to supercooled liquids [1]. 1T-TaS<sub>2</sub>, a layered dichalcogenide, is a unique platform for studying dynamic phase transitions in quantum materials [2]. Upon quenching 1T-TaS<sub>2</sub> after excitation with an ultrafast laser pulse, a low-temperature metallic metastable phase (H-CDW) emerges [3], which is different from any of the charge density wave (CDW) phases characterizing its thermodynamic phase diagram. I will show that a new metastable insulating phase with similar scattering signatures to the H-CDW [4] can be stabilized by intermediate quenching rates [5]. I will discuss the implications of this new phase in the controversy surrounding the presence of Mott physics and the role of c-axis correlations [6] in the equilibrium ground state of 1T-TaS<sub>2</sub>.<br/><br/>[1] Zhiyuan Sun and Andrew J. Millis Phys. Rev. X 10, 021028 (2020)<br/>[2] B. Sipos et al., Nat. Mat. 7, 960 (2008)<br/>[3] L. Stojchesvka et al., Science 344, 177 (2014)<br/>[4] Stahl et al., Nat. Commun. 11, 1247 (2020)<br/>[5] AdlT et al., in preparation<br/>[6] S-H Lee et al., PRL 122, 106404 (2019)

Keywords

metal-insulator transition

Symposium Organizers

Ajay Ram Srimath Kandada, Wake Forest University
Nicolò Maccaferri, Umeå University
Chiara Trovatello, Columbia University
Ursula Wurstbauer, Technical University of Munich

Symposium Support

Bronze
LIGHT CONVERSION

Publishing Alliance

MRS publishes with Springer Nature