MRS Meetings and Events

 

EN02.03.16 2022 MRS Fall Meeting

In Situ Core/Shell Perovskites for Ultra-Bright, Efficient and Stable Light-Emitting Diodes

When and Where

Nov 28, 2022
8:00pm - 10:00pm

Hynes, Level 1, Hall A

Presenter

Co-Author(s)

Joo Sung Kim1,Jung-Min Heo1,Gyeong-Su Park1,Seung-Je Woo1,Changsoon Cho2,Hyung Joong Yun3,Dong-Hyeok Kim1,Jinwoo Park1,Seung-Chul Lee1,Sang-Hwan Park1,Eojin Yoon1,Neil Greenham2,Tae-Woo Lee1

Seoul National University1,University of Cambridge2,Korea Basic Science Institute3

Abstract

Joo Sung Kim1,Jung-Min Heo1,Gyeong-Su Park1,Seung-Je Woo1,Changsoon Cho2,Hyung Joong Yun3,Dong-Hyeok Kim1,Jinwoo Park1,Seung-Chul Lee1,Sang-Hwan Park1,Eojin Yoon1,Neil Greenham2,Tae-Woo Lee1

Seoul National University1,University of Cambridge2,Korea Basic Science Institute3
Metal halide perovskites are attracting great attention as next-generation light-emitting materials due to their excellent emission properties with narrowband emission. However, perovskite light-emitting diodes (PeLEDs) irrespective of their material types (polycrystalline film or nanocrystals) have not realized high luminance, high efficiency, and long lifetime simultaneously, as they are influenced by the intrinsic limitations related to the trade-off properties between charge transport and confinement in each type of perovskite materials. Here, we report bright, efficient, and stable PeLEDs made of core/shell perovskite nanocrystals obtained using a simple <i>in-situ</i> reaction. The ligand passivates the surface defect states, and thereby greatly reduces trap density in films while maintaining good charge-transport properties. Our work sheds great light on the possibility that PeLEDs can be commercialized in the future display industry.

Keywords

grain size | perovskites

Symposium Organizers

Jin-Wook Lee, Sungkyunkwan University
Carolin Sutter-Fella, Lawrence Berkeley National Laboratory
Wolfgang Tress, Zurich University of Applied Sciences
Kai Zhu, National Renewable Energy Laboratory

Symposium Support

Bronze
ACS Energy Letters
ChemComm
MilliporeSigma
SKKU Insitute of Energy Science & Technology

Session Chairs

Il Jeon
Jin-Wook Lee
Carolin Sutter-Fella
Wolfgang Tress

In this Session

EN02.03.01
Rational Design of Photoelectrochemical Perovskite-BiVO4 Tandem Devices for Scalable Solar Fuel Production

EN02.03.02
Mechanochemistry-Driven Engineering of Cs4PbX6/CsPbX3 (X=Cl, Br, I) Heterostructure for Designing Highly Luminescent Perovskites

EN02.03.03
Entirely Roll to Roll Coated Perovskite Photovoltaics Enabled by Carbon Ink Formulation

EN02.03.04
Morphology-Controlled Lead-Free Halide Double Perovskite Nanocrystals by Chemical Vapor Deposition

EN02.03.05
3D Printing of Ruddlesden-Popper Perovskites with High Color Purity and Stability

EN02.03.07
Perovskite and Organic Photoanodes with Low-Temperature Printed Carbon Layer for Solar Water Splitting

EN02.03.09
Co-Evaporation and Characterization of Tin Based Perovskite Films For Solar Cell Applications

EN02.03.10
Hierarchically Ordered Perovskites with High Photo-Electronic and Environmental Stability via Nanoimprinting Guided Block Copolymer Self-Assembly

EN02.03.11
Air and Oxygen Stable Core/Shell Perovskite Nanocrystals for Deep-Blue LED Application

EN02.03.12
Lighting Beyond Blue—Violet Metal Halide Perovskite Light-Emitting Diodes

View More »

Publishing Alliance

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