April 22 - 26, 2024
Seattle, Washington
May 7 - 9, 2024 (Virtual)

Event Supporters

2024 MRS Spring Meeting
CH04.10.02

Novel Electrical Tree Type Observed using Gigahertz Frame Rate Camera to Image Dielectric Breakdown in Space-Charged Polymer

When and Where

Apr 26, 2024
8:15am - 8:30am
Room 443, Level 4, Summit

Presenter(s)

Co-Author(s)

Kathryn Sturge1,Noah Hoppis1,Ariana Bussio1,Jonathan Barney2,Brian Beaudoin1,Cameron Brown2,Bruce Carlsten2,Carolyn Chun1,Nicholas Dallmann2,Jack Fitzgibbon1,Ashley Hammell1,Samuel Henderson2,Miriam Hiebert1,James Krutzler1,Joseph Lichthardt2,Mark Marr-Lyon2,Nathan Moody2,Alexander Mueller2,Patrick O'Shea1,Ryan Schneider1,Karl Smith2,Bryce Tappan2,Clayton Tiemann2,David Walter2,Timothy Koeth1

University of Maryland, College Park1,Los Alamos National Laboratory2

Abstract

Kathryn Sturge1,Noah Hoppis1,Ariana Bussio1,Jonathan Barney2,Brian Beaudoin1,Cameron Brown2,Bruce Carlsten2,Carolyn Chun1,Nicholas Dallmann2,Jack Fitzgibbon1,Ashley Hammell1,Samuel Henderson2,Miriam Hiebert1,James Krutzler1,Joseph Lichthardt2,Mark Marr-Lyon2,Nathan Moody2,Alexander Mueller2,Patrick O'Shea1,Ryan Schneider1,Karl Smith2,Bryce Tappan2,Clayton Tiemann2,David Walter2,Timothy Koeth1

University of Maryland, College Park1,Los Alamos National Laboratory2
We have successfully imaged dielectric breakdown occurring in electron irradiated space-charged polymethyl methacrylate (PMMA) blocks at a nanosecond time resolution. These images, which are the first of their kind, reveal two distinct dielectric breakdown treeing effects, one of which is absent from the present literature on dielectric breakdown. This new mode of electrical tree formed during dielectric breakdown of a space-charged polymer demonstrates unique behavior from its better-documented and widely known “branch-type” channels, including structural and formation dynamics differences. Due to its threadlike, smooth appearance, this new type of electrical tree has been coined “vine-type,” in contrast to its “branch-type” counterpart. Both vine-type and branch-type electrical trees were imaged as they formed in the electron irradiated samples, allowing for close study of the channel formation dynamics. The speeds at which the channels form for both types were directly measured from these images and found to exceed 10<sup>7</sup> m/s and 10<sup>6</sup> m/s for vine-type and branch-type, respectively—speeds approaching 4% the speed of light in the material. These speeds are faster than previously predicted by models and imply the channel growth is the fastest physical phenomenon in a solid material. Further, the propagation of the electrical tree formation was imaged and three regimes of breakdown channel formation were identified and characterized for the two modes of electrical trees, solving a decades-long mystery on the plasma channel formation process in space-charge dielectric breakdown.

Keywords

dielectric properties

Symposium Organizers

Yuzi Liu, Argonne National Laboratory
Michelle Mejía, Dow Chemical Co
Yang Yang, Brookhaven National Laboratory
Xingchen Ye, Indiana University

Session Chairs

Tianyi Li
Michelle Mejía
Yang Yang

In this Session