December 1 - 6, 2024
Boston, Massachusetts

Event Supporters

2024 MRS Fall Meeting & Exhibit
QT05.02.02

Disorder- and Interaction-Dominated Quantum Criticalities in WSe2

When and Where

Dec 2, 2024
2:00pm - 2:15pm
Sheraton, Fifth Floor, Riverway

Presenter(s)

Co-Author(s)

Nasir Ali1,Fida Ali2,Hyungyu Choi1,Inhee Jeong1,Hyokwang Park1,Hoseong Shin1,Kwangro Lee1,Zhipei Sun2,Won Jong Yoo1

Sungkyunkwan University1,Aalto University2

Abstract

Nasir Ali1,Fida Ali2,Hyungyu Choi1,Inhee Jeong1,Hyokwang Park1,Hoseong Shin1,Kwangro Lee1,Zhipei Sun2,Won Jong Yoo1

Sungkyunkwan University1,Aalto University2
Quantum fluctuations owing to strong Coulomb interactions or strong disorder lead to quantum phase transition (QPT) in 2D systems. However, understanding of disorder- and interaction-driven QPTs remains a fundamental challenge in condensed matter physics. Here, we use thickness-dependent WSe<sub>2</sub> to elucidate the quantum phase metal-insulator transition driven by strong disorder, and strong Coulomb interactions in thin- and thick-WSe<sub>2</sub>, respectively. An observation of crossover conductance ~e<sup>2</sup>/<i>h</i> signifies the role of quantum fluctuations due to strong disorder in bi- and five-layer WSe<sub>2</sub>. In contrary, the crossover conductance ~0.1 e<sup>2</sup>/<i>h</i> demonstrates bad-metal behavior associated with Mott quantum criticality owing to strong Coulomb interactions in ten-layer WSe<sub>2</sub>. In the metallic phase, resistivity (<i>ρ</i>) follows Fermi-liquid (<i>ρ</i> ∝ <i>T</i><sup>2</sup>) and non-Fermi-liquid (<i>ρ</i> ∝ <i>T</i><sup>1.5</sup>) behaviors in bi- and five-layer WSe<sub>2</sub> from low to high temperatures, respectively. In ten-layer WSe<sub>2</sub>, <i>ρ </i>displays a <i>T</i><sup>2</sup>-dependence at low temperatures while it shows a <i>T-</i>linear behavior at moderate temperatures in the deep metallic phase, suggestive of strange-metal behavior. Further, the strange-metal transforms into the bad-metal around the crossover point in ten-layer WSe<sub>2</sub>. Moreover, conductivity (<i>σ</i>) exhibits a <i>T</i>-dependence as δ<i>σ</i> ∝ <i>T</i><sup>3/2</sup> in the vicinity of critical point, suggesting the metallic glass phase which highlights the significant role of strong disorder and Coulomb interactions in bi- and five-layer WSe<sub>2</sub> devices. The absence of such a phase in ten-layer WSe<sub>2</sub> attributes that the Coulomb interactions dominate over disorder in ten-layer WSe<sub>2</sub>. Critical scaling of conductivity as a function of temperature and carrier density reveals the disorder-dominated quantum criticality in bi- and five-layer WSe<sub>2</sub>, and interaction-dominated quantum criticality in ten-layer WSe<sub>2</sub>. This study provides compelling evidence that thickness-dependent WSe<sub>2</sub> serves as a new platform to study the disorder- and interaction-dominated QPTs in 2D systems.

Keywords

2D materials | metal-insulator transition

Symposium Organizers

Annabelle Bohrdt, Universität Regensburg
Paola Cappellaro, Massachusetts Institute of Technology
Avetik Harutyunyan, Honda Research Institute USA Inc
Yao Wang, Emory University

Symposium Support

Silver
Honda Research Institute USA Inc.

Session Chairs

Annabelle Bohrdt
Yu He

In this Session