December 1 - 6, 2024
Boston, Massachusetts

Event Supporters

2024 MRS Fall Meeting & Exhibit
NM05.03.05

Selective Spin-Triplet and Spin-Singlet Interlayer Exciton Emission in WS2/WSe2 Heterostructure for All-Optical Valley Switch

When and Where

Dec 2, 2024
11:30am - 11:45am
Hynes, Level 2, Room 207

Presenter(s)

Co-Author(s)

Yue Hu1,Xinglin Wen1,Dehui Li1

Huazhong University of Science & Technology1

Abstract

Yue Hu1,Xinglin Wen1,Dehui Li1

Huazhong University of Science & Technology1
Spin-splitting in transition metal dichalcogenides (TMDs) heterostructure generate spin-singlet and spin-triplet interlayer exciton (IX) with unique spin-valley physics. Although selective singlet and triplet IX emission can be achieved by applying electric<sup> </sup>and magnetic<sup> </sup>field, the device structure is complex and low-temperature condition is demanding. Here, by selectively coupling singlet or triplet IX dipole of WS<sub>2</sub>/WSe<sub>2</sub> heterostructure to a SiO<sub>2</sub> sphere cavity, we can actively control the emissive IX species at room temperature in an all-optical route. We find the triplet IX dipole is almost along the out-of-plane orientation, whereas, only 69% of the singlet IX dipole is out-of-plane. Consequently, triplet IX emission is enhanced more greatly in TMDs/SiO<sub>2</sub> cavity hybrid structure due to that out-of-plane dipole presents higher Purcell factor for SiO<sub>2</sub> cavity. By utilizing the selective enhancement of singlet and triplet IX emission, we demonstrated an all-optical valley switch. Our finding provides a convenient approach to control the fine structure of IX and develop their applications in valleytronics.

Keywords

2D materials | spin

Symposium Organizers

Andras Kis, Ecole Polytechnique Federale de Lausanne
Li Lain-Jong, University of Hong Kong
Ying Wang, University of Wisconsin, Madison
Hanyu Zhu, Rice University

Session Chairs

Xiao-Xiao Zhang
Hanyu Zhu

In this Session